numerical analysis of the optimal catalyst distribution in created unsteady state conditions
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abstract
the determination of the optimal distribution of the catalytic activity profile, whichmaximizes the catalytic effectiveness, in created unsteady state conditions, is analyzed andtreated numerically for the case of a simple reaction. it was proven that the modulation, of thetemperature and the reactant concentration of the external bulk fluid, leads to a considerableincrease of the catalytic effectiveness. the optimal active element distribution is a dirac- δfunction i.e. all the catalyst must be deposited at a specific distance from the center of thecatalytic pellet. it was shown that this optimal position changes with time in a sinusoidal manner.this purpose can be achieved by the use of ultrasounds to artificially control the activity profile.
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Journal title:
journal of the iranian chemical researchجلد ۲، شماره ۲، صفحات ۱۲۱-۱۳۱
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